eT

eT is a quantum chemistry program specialized in calculating molecular response properties and time-dependent phenomena using coupled cluster theory. Developed with focus on response properties, excited states, and spectroscopic calculat…

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Overview

eT is a quantum chemistry program specialized in calculating molecular response properties and time-dependent phenomena using coupled cluster theory. Developed with focus on response properties, excited states, and spectroscopic calculations, eT implements efficient coupled cluster methods with particular emphasis on equations-of-motion and linear response approaches for accurate molecular properties.

Reference Papers (1)

Full Documentation

Official Resources

  • Homepage: https://etprogram.org/
  • Documentation: https://etprogram.org/user_manual.html
  • Source Repository: https://gitlab.com/eT-program/eT
  • License: GNU General Public License v3.0

Overview

eT is a quantum chemistry program specialized in calculating molecular response properties and time-dependent phenomena using coupled cluster theory. Developed with focus on response properties, excited states, and spectroscopic calculations, eT implements efficient coupled cluster methods with particular emphasis on equations-of-motion and linear response approaches for accurate molecular properties.

Scientific domain: Coupled cluster, response properties, excited states, spectroscopy
Target user community: Spectroscopy researchers, response property calculations, CC method users

Theoretical Methods

  • Coupled cluster (CC2, CCSD, CC3)
  • Equations-of-motion coupled cluster (EOM-CC)
  • Linear response coupled cluster
  • Time-dependent coupled cluster
  • Hartree-Fock
  • Response properties
  • Excited states
  • Transition properties
  • Spectroscopic properties

Capabilities (CRITICAL)

  • Ground-state coupled cluster
  • Excited states (EOM-CC)
  • Response properties
  • Molecular properties
  • Spectroscopic calculations
  • Transition moments
  • Oscillator strengths
  • UV/Vis spectra
  • Linear response
  • Time-dependent properties
  • High-accuracy calculations
  • Research-quality results

Sources: Official website (https://etprogram.org/)

Key Strengths

Response Properties:

  • Specialized focus
  • CC response theory
  • Accurate properties
  • Transition moments
  • Spectroscopic data

Coupled Cluster:

  • CC2, CCSD, CC3
  • EOM-CC for excitations
  • High accuracy
  • Benchmark quality
  • Production methods

Spectroscopy:

  • UV/Vis calculations
  • Excitation energies
  • Oscillator strengths
  • Transition properties
  • Experimental comparison

Open Source:

  • GPL v3 licensed
  • GitLab repository
  • Free to use
  • Community development
  • Transparent code

Research Tool:

  • Method development
  • Property calculations
  • Benchmark studies
  • Accurate results
  • Academic focus

Inputs & Outputs

  • Input formats:

    • Text-based input
    • Molecular coordinates
    • Basis set specifications
    • Method settings
  • Output data types:

    • Energies
    • Excitation energies
    • Properties
    • Transition moments
    • Spectroscopic data

Interfaces & Ecosystem

  • Development:

    • GitLab repository
    • Community contributions
    • Research tool
  • Analysis:

    • Property extraction
    • Spectroscopy analysis
    • Standard tools
    • Custom scripts

Workflow and Usage

Typical Workflow:

  1. Prepare molecular structure
  2. Select CC method
  3. Choose basis set
  4. Configure response properties
  5. Run eT calculation
  6. Analyze results

Running eT:

et input.inp
# Runs coupled cluster calculation

Advanced Features

EOM-CC:

  • Equations-of-motion
  • Excited states
  • Accurate excitations
  • Multiple states
  • Transition properties

Response Theory:

  • Linear response
  • Time-dependent properties
  • Molecular properties
  • Spectroscopic calculations
  • High accuracy

CC Methods:

  • CC2 (approximate)
  • CCSD (standard)
  • CC3 (high accuracy)
  • Gradients (selected)
  • Production quality

Performance Characteristics

  • Speed: Moderate (high-level CC)
  • Accuracy: Excellent for properties
  • System size: Small to medium molecules
  • Scalability: Typical CC scaling
  • Typical: Research calculations

Computational Cost

  • CC2: Moderate cost
  • CCSD: Expensive
  • CC3: Very expensive
  • Response: Additional cost
  • Production: Research-level feasible

Limitations & Known Constraints

  • System size: Limited by CC scaling
  • Community: Smaller, specialized
  • Documentation: Research-level
  • Features: Focused on properties
  • Platform: Linux primarily
  • Development: Academic/research

Comparison with Other Codes

  • vs CFOUR: eT specialized for response properties
  • vs Dalton: Similar focus, different implementation
  • vs PSI4: eT more specialized
  • Unique strength: CC response properties, EOM-CC, spectroscopy focus

Application Areas

Spectroscopy:

  • UV/Vis calculations
  • Excitation energies
  • Transition moments
  • Oscillator strengths
  • Experimental comparison

Response Properties:

  • Molecular properties
  • Linear response
  • Time-dependent
  • High accuracy
  • Benchmark calculations

Excited States:

  • EOM-CC calculations
  • Multiple states
  • Accurate excitations
  • State properties
  • Transition densities

Method Development:

  • CC response research
  • Algorithm testing
  • Benchmark studies
  • Property methods

Best Practices

Method Selection:

  • CC2 for screening
  • CCSD for production
  • CC3 for benchmarks
  • Appropriate for system
  • Balance accuracy/cost

Basis Sets:

  • Appropriate for properties
  • Augmented when needed
  • Convergence testing
  • Balance size/accuracy

Response Calculations:

  • Select properties carefully
  • Converge SCF well
  • Check stability
  • Validate results

Community and Support

  • Open-source (GPL v3)
  • GitHub repository
  • Academic development
  • Research community
  • Limited production support

Educational Resources

  • GitHub documentation
  • Source code
  • Published papers
  • CC theory literature
  • Response property references

Development

  • GitHub-based development
  • Academic contributors
  • Research focus
  • Ongoing improvements
  • Community input

Research Applications

  • Response property calculations
  • Spectroscopy predictions
  • Benchmark studies
  • Method development
  • High-accuracy properties

Technical Innovation

CC Response:

  • Efficient implementations
  • Response theory
  • Property calculations
  • Specialized algorithms
  • Research quality

EOM-CC:

  • Excited state methods
  • Accurate excitations
  • Transition properties
  • Multiple states
  • Production implementations

Verification & Sources

Primary sources:

  1. Official website: https://etprogram.org/
  2. Documentation: https://etprogram.org/user_manual.html
  3. GitLab repository: https://gitlab.com/eT-program/eT
  4. Published papers on eT methodology

Secondary sources:

  1. Coupled cluster literature
  2. Response property methods
  3. EOM-CC references
  4. Spectroscopy calculations

Confidence: LOW_CONF - Research code, specialized focus, smaller community

Verification status: ✅ VERIFIED

  • Official website: ACCESSIBLE (https://etprogram.org/)
  • Documentation: ACCESSIBLE (user manual)
  • Source code: OPEN (GitLab, GPL v3)
  • Community support: GitLab, academic
  • Development: Active on GitLab
  • Specialized strength: Coupled cluster response properties, EOM-CC excited states, spectroscopic calculations, molecular properties, linear response theory, benchmark-quality accuracy

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