COHP

**Status**: METHOD/TOOL - COHP refers to the Crystal Orbital Hamilton Population method, a theoretical framework for analyzing chemical bonding in solids by partitioning the band structure energy into bonding and antibonding contribution…

8. POST-PROCESSING 8.4 Chemical Bonding Analysis VERIFIED 1 paper
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Overview

**Status**: METHOD/TOOL - COHP refers to the Crystal Orbital Hamilton Population method, a theoretical framework for analyzing chemical bonding in solids by partitioning the band structure energy into bonding and antibonding contributions. While "COHP" is a method, the term is often used to refer to the LOBSTER code (which implements it) or legacy codes like Cray-COHP.

Reference Papers (1)

Full Documentation

Official Resources

  • Homepage: https://www.cohp.de/
  • Documentation: http://www.cohp.de/
  • Source Repository: Part of LOBSTER or other implementations
  • License: Varies (LOBSTER is academic free)

Overview

Status: METHOD/TOOL - COHP refers to the Crystal Orbital Hamilton Population method, a theoretical framework for analyzing chemical bonding in solids by partitioning the band structure energy into bonding and antibonding contributions. While "COHP" is a method, the term is often used to refer to the LOBSTER code (which implements it) or legacy codes like Cray-COHP.

Scientific domain: Chemical bonding analysis, solid-state chemistry
Target user community: Solid-state chemists, materials scientists

Theoretical Methods

  • Partitioning of band structure energy
  • Bonding/Antibonding analysis
  • Projected density of states (pDOS)
  • Crystal Orbital Overlap Population (COOP)
  • Integrated COHP (ICOHP) for bond strength

Capabilities (CRITICAL)

  • Visualization of bonding interactions (bonding vs. antibonding)
  • Quantitative assessment of bond strengths (ICOHP)
  • Analysis of electronic stability
  • Implemented in: LOBSTER (standard), tight-binding codes, some DFT packages (SIESTA, LMTO)

Sources: Dronskowski and Bloechl, J. Phys. Chem. 97, 8617 (1993)

Key Strengths

Chemical Insight:

  • Direct bonding/antibonding visualization
  • Energy-resolved analysis
  • Quantitative ICOHP values
  • Intuitive interpretation

Solid-State Focus:

  • Designed for crystals
  • Periodic boundary support
  • Band structure connection
  • Extended systems

Wide Implementation:

  • LOBSTER (primary)
  • SIESTA/LMTO codes
  • Academic standard
  • Well-documented theory

Inputs & Outputs

  • Input: Wavefunctions/Hamiltonians from DFT (VASP, QE, etc.)
  • Output: COHP vs Energy plots, ICOHP values

Interfaces & Ecosystem

  • LOBSTER: The main modern implementation
  • LobsterPy: Python analysis tool
  • VASP/QE: Source of electronic structure data

Limitations & Known Constraints

  • Projection dependent: Results depend on local basis choice
  • Not unique: Different projections give different COHP
  • Interpretation: Requires chemical knowledge
  • Implementation: Mainly via LOBSTER for plane-wave codes

Comparison with Other Tools

  • vs COOP: COHP energy-weighted, COOP overlap-weighted
  • vs Bader: COHP bonding analysis, Bader charge partitioning
  • vs ELF: Different perspectives on bonding
  • Unique strength: Direct bonding/antibonding energy analysis

Application Areas

  • Phase stability analysis
  • Magnetic ordering origins
  • Bond strength in intermetallics
  • Surface adsorption

Best Practices

  • Use adequate k-point sampling
  • Choose appropriate energy window
  • Compare ICOHP values for bond strength ranking
  • Validate with known compounds

Verification & Sources

Primary sources:

  1. Homepage: https://www.cohp.de/
  2. Publication: R. Dronskowski, P. E. Bloechl, J. Phys. Chem. 97, 8617 (1993)

Confidence: VERIFIED

Verification status: ✅ VERIFIED

  • Method: STANDARD
  • Implementation: Primarily via LOBSTER
  • Applications: Bonding analysis

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