TopMod

TopMod is a FORTRAN package for topological analysis of the Electron Localization Function (ELF). It calculates the ELF on a 3D grid, assigns basins, and computes basin populations and their variances. This enables quantitative analysis…

8. POST-PROCESSING 8.4 Chemical Bonding Analysis VERIFIED
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Overview

TopMod is a FORTRAN package for topological analysis of the Electron Localization Function (ELF). It calculates the ELF on a 3D grid, assigns basins, and computes basin populations and their variances. This enables quantitative analysis of chemical bonding in terms of core, bonding, and lone pair basins.

Reference Papers

Reference papers are not yet linked for this code.

Full Documentation

Official Resources

  • Homepage: https://www.lct.jussieu.fr/pagesperso/silvi/topmod_english.html
  • Documentation: https://www.lct.jussieu.fr/pagesperso/fuster/TOPMOD/topmod-manual.pdf
  • Source: Available from homepage
  • License: Academic use

Overview

TopMod is a FORTRAN package for topological analysis of the Electron Localization Function (ELF). It calculates the ELF on a 3D grid, assigns basins, and computes basin populations and their variances. This enables quantitative analysis of chemical bonding in terms of core, bonding, and lone pair basins.

Scientific domain: ELF topology, chemical bonding, electron localization Target user community: Researchers studying chemical bonding through electron localization

Theoretical Methods

  • Electron Localization Function (ELF)
  • Topological analysis (gradient field)
  • Basin assignment and integration
  • Population and variance calculation
  • Synaptic order classification

Capabilities (CRITICAL)

  • ELF Calculation: 3D grid evaluation
  • Basin Analysis: Core, bonding, lone pair basins
  • Population: Basin electron populations
  • Variance: Population fluctuation analysis
  • Synaptic Order: Basin connectivity
  • Visualization: Basin boundaries

Sources: TopMod documentation, Silvi group publications

Key Strengths

ELF Specialization:

  • Complete ELF analysis
  • Basin classification
  • Population statistics
  • Quantitative bonding

Established Method:

  • Well-validated
  • Extensive literature
  • Standard methodology
  • Benchmark results

Gaussian Compatible:

  • Direct wfn input
  • Standard format support
  • Easy workflow
  • Gaussian 92-16

Inputs & Outputs

  • Input formats:

    • Gaussian wfn files
    • Standard wavefunction format
  • Output data types:

    • ELF values on grid
    • Basin assignments
    • Population values
    • Variance statistics

Installation

# Download from homepage
tar -xvf topmod.tar
cd topmod
make

Usage Examples

# Prepare input file
# Run TopMod
./topmod < input.dat

# Input file format:
molecule.wfn    # wavefunction file
80 80 80        # grid points
0.1             # step size

Performance Characteristics

  • Speed: Efficient grid evaluation
  • Memory: Depends on grid size
  • Accuracy: Well-established method

Limitations & Known Constraints

  • FORTRAN: Older codebase
  • Grid-based: Resolution dependent
  • Documentation: Limited online resources
  • Visualization: Requires external tools

Comparison with Other Tools

  • vs Multiwfn: TopMod specialized ELF, Multiwfn broader
  • vs Critic2: TopMod ELF focus, Critic2 general topology
  • vs DGrid: Different ELF implementations
  • Unique strength: Original ELF topology implementation

Application Areas

  • Chemical bond characterization
  • Lone pair identification
  • Hypervalent bonding
  • Metallic bonding analysis
  • Electron pair domains

Best Practices

  • Use sufficient grid resolution
  • Verify basin connectivity
  • Compare populations with expectations
  • Cross-validate with other methods

Community and Support

  • LCT Paris group
  • Academic distribution
  • Published methodology
  • Bernard Silvi (developer)

Verification & Sources

Primary sources:

  1. Homepage: https://www.lct.jussieu.fr/pagesperso/silvi/topmod_english.html
  2. S. Noury et al., Comput. Chem. 23, 597 (1999)
  3. B. Silvi, A. Savin, Nature 371, 683 (1994)

Confidence: VERIFIED - Established academic software

Verification status: ✅ VERIFIED

  • Homepage: ACCESSIBLE
  • Documentation: AVAILABLE (PDF)
  • Source code: ACADEMIC distribution
  • Developer: Bernard Silvi (LCT Paris)
  • Academic citations: Well-cited
  • Method: ELF topology analysis

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